Balloon AirCore Data Tightens Estimates of Stratospheric Methane and Carbonyl Sulfide Lifetimes
bioengineer.orgResearchers used balloon-borne AirCore samplers to measure vertical profiles of carbonyl sulfide and methane in the lower stratosphere. The study, published in Atmospheric Chemistry and Physics, compares those profiles with nitrous oxide as a reference tracer. It estimates a stratospheric lifetime of about 76 years for carbonyl sulfide and roughly 150 to 166 years for methane. Those numbers are consistent with satellite observations and help reduce uncertainty in how these gases are removed from the atmosphere. AirCore is a coiled steel tube that collects air during descent, then gets analyzed with laser spectroscopy on the ground. The approach gives higher vertical resolution than satellite remote sensing and is cheaper to repeat. The authors also found no significant long-term trend in stratospheric removal rates, which means changes in methane and carbonyl sulfide burdens are driven mainly by emissions and transport. Tighter lifetime estimates matter for climate modeling and for methane policy. If the stratospheric sink is steady, observed methane growth points back to rising emissions. That makes atmospheric measurements like these useful for verifying emission inventories and tracking progress on reduction commitments.
